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Study On Removing NO_x By Plasma Assisted Low Temperature Catalyst

Posted on:2017-06-14Degree:MasterType:Thesis
Country:ChinaCandidate:Y D PengFull Text:PDF
GTID:2321330563950604Subject:Optical Engineering
Abstract/Summary:PDF Full Text Request
Nitrogen oxides is not only the culprit of the formation of such as acid rain and mist,but the emissions of nitrogen oxides also take place secondary reaction and produce second aerosol pollutants in the atmosphere,which is one of the reasons for the formation of haze.So to improve the removal efficiency of NOx and reduce the energy consumption of the NOx removal is currently one of the focuses of the study.Plasma has been widely used in waste gas.The removal of flue gas pollutants by plasma has good effect,no second pollution,simultaneously removing various pollutants and so on.This experiment remove NOx by the plasma assisted low-temperature SCR catalyst,by changing the gas composition in simulated flue gas studying the effects on catalytic effect with adding different additives.In addition,The experiment has compared with the synergistic effect of PDC?Plasma-Driven Catalysis?and PEC?Plasma-Enhanced Catalysis?s in the same conditions,and the addition of C2H4 in the simulated flue gas has different effect.The MnOx-CeO2-V2O5/TiO2 catalyst is prepared with low-temperature catalytic effect according to a certain proportion.It can effectively reduce the catalytic temperature of NOx removal and improve the catalytic removal efficiency.Using PDC for a layout and studying on the effects of different atmosphere on concerted catalysis.Results show that the removal effect of NOx by individual plasma is relatively poor and with high energy consumption.But Plasma synergistic catalysis can obviously enhance the removal efficiency of NOx,and reduce the energy consumption of the plasma.To improve the removal efficiency of NOx is low only with ammonia in the simulated flue gas,while adding ethylene has only increased the yield of NO2 and has almost no effect on the removal of NOx.But withing NH3 and C2H4 at the same time in the simulated flue gas,the conversion rate of NO greatly increased at 100 in the case and almost completely transformed,and the removal efficiency of NOx is greatly increased,and greatly reducing NOx removal temperature.To compare the two catalytic form of PDC and PEC under the same conditions,it is found that plasma driven catalytic form has higher removal efficiency at the same temperature and energy consumption,and the effect is more obvious in the case of the accession of C2H4 and NH3.
Keywords/Search Tags:Plasma, Low temperature SCR de-NO_x catalyst, Plasma-Driven Catalysis, Plasma-Enhanced Catalysis, De-NO_x, Synergistic catalysis
PDF Full Text Request
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