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Transport in Weakly Coupled Vertical Double Quantum Dots: Single-Particle Energy Level Spectroscopy and Hyperfine Interaction Effects

Posted on:2012-10-18Degree:Ph.DType:Dissertation
University:McGill University (Canada)Candidate:Payette, ChristopherFull Text:PDF
GTID:1460390011959431Subject:Physics
Abstract/Summary:
Performing transport measurements on weakly coupled vertical double quantum dots, we study by magneto-resonant-tunneling spectroscopy, single-particle energy spectra of the constituent dots over a wide energy window. The measured energy spectra are well modeled overall by ideal spectra calculated for elliptical and parabolic in-dot-plane confinement potentials. However, in regions where single-particle energy levels are naively expected to cross, we observe pronounced level anti-crossing behaviour and strong resonant current variations (both enhancement and suppression). Within a coherent tunneling picture, these effects can be attributed to coherent level mixing induced by weak perturbations in the nearly ideal dot confinement potentials. We analyze the energy spectra in detail, and focus on examples of two-, three- and four-level crossings where we observe the suppression of an otherwise strong current resonance, a signature of dark state formation due to destructive interference. The mixing we measure and model at two three-level crossings represents an all-electrical analogue of coherent population trapping. We also explore the limitations of the applicability of the coherent level mixing model and demonstrate in-situ alteration of the coupling between levels.;We further examine the electron spin-nuclear spin (hyperfine) interaction. In the familiar two-electron spin blockade regime, on application of an out-of-dot-plane magnetic field, we observe current switching and hysteresis, and a funnel-like structure in the leakage current, all hallmarks of the hyperfine interaction. The measurements bring to light a strong gate voltage dependence, significant device-to-device variations, and an intricate bias voltage history dependence not accounted for in any existing model. Unexpectedly, we also observe signatures of the hyperfine interaction at high bias, well outside the spin blockade regime. We characterize these features and suggest how the hyperfine interaction may play a role at high bias, although the electronic states involved generally can not easily be identified. As a first step toward understanding this new regime, we describe another hysteretic funnel-like structure observed at high bias where the electronic states involved can be identified as two-electron states, so allowing us to postulate a specific mechanism for this funnel.
Keywords/Search Tags:Single-particle energy, Hyperfine interaction, Dots, Level
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